Chris Evans
Steve Rogers / Captain America
Samuel L. Jackson
Nick Fury
Scarlett Johansson
Natasha Romanoff / Black Widow
Robert Redford
Alexander Pierce
Sebastian Stan
Bucky Barnes / Winter Soldier
Anthony Mackie
Sam Wilson / Falcon
Maximiliano Hernández
Jasper Sitwell
Emily VanCamp
Kate / Agent 13
Hayley Atwell
Peggy Carter
Stan Lee
Smithsonian Guard
Callan Mulvey
Jack Rollins
Jenny Agutter
Councilwoman Hawley
Bernard White
Councilman Singh
Alan Dale
Councilman Rockwell
Garry Shandling
Senator Stern
Georges St-Pierre
Georges Batroc
Salvator Xuereb
French Pirate #1
Brian Duffy
French Pirate #2
Adetokumboh M'Cormack
French Radio Pirate
Christopher George Sarris
Skinny Steve
Aaron Himelstein
Launch Tech #1
Allan Chanes
Launch Tech #2
Christopher Markus
SHIELD Interrogator #1
Stephen McFeely
SHIELD Interrogator #2
D.C. Pierson
Apple Employee
Bernie Zilinskas
Com Tech #2
Angela Russo-Otstot
Garcia
Chad Todhunter
Charlie Weapons Tech
Abigail Marlowe
SHIELD Tech
Jeremy Maxwell
Lead SHIELD Pilot
Emerson Brooks
Senior SHIELD Agent
Ricardo Chacon
Strike SGT. #1
Griffin M. Allen
Strike SGT. #2
Michael Debeljak
Strike Agent
Eddie J. Fernandez
Strike Agent
Jody Hart
25ᵗʰ Floor Strike Agent
Derek Hughes
Human Resources Executive
Dominic Rains
CIA Instructor
Charles Wittman
Capitol Hill Police
Andy Martinez, Jr.
Capitol Hill Police
Terence O'Rourke
FBI Agent
Anne Grimenstein
Committee Member
Dante Rosalina
Little Boy in the Smithsonian
Robert Clotworthy
Fury Car Voice (voice)
June Christopher
SHIELD Computer (voice)
Gary Sinise
The Smithsonian Narrator (voice)
Henry Goodman
Dr. List (uncredited)
Dean Barlage
SHIELD Agent (uncredited)
Joel Thingvall
Museum Visitor (uncredited)
Thomas Kretschmann
Baron Wolfgang von Strucker (uncredited)
Elizabeth Olsen
Wanda Maximoff / Scarlet Witch (uncredited)
Nestor Serrano
Committee General (uncredited)
Aaron Taylor-Johnson
Pietro Maximoff / Quicksilver (uncredited)
Joss Whedon
Man on Escalator in Museum (uncredited)