All Cast

Jack Angel

Jack Angel

Papa Smurf (voice)

Fred Armisen

Fred Armisen

Brainy (voice)

Hank Azaria

Hank Azaria

Gargamel (voice)

Gary Basaraba

Gary Basaraba

Hefty (voice)

George Lopez

George Lopez

Grouchy (voice)

Melissa Sturm

Melissa Sturm

Smurfette (voice)

Anton Yelchin

Anton Yelchin

Clumsy (voice)

Frank Welker

Frank Welker

Azrael (voice)

Kirk Baily

Kirk Baily

Additional Voices (voice)

Jess Harnell

Jess Harnell

Additional Voices (voice)

Jeff Fischer

Jeff Fischer

Additional Voices (voice)

Craig Kellman

Craig Kellman

Additional Voices (voice)

John Hans Tester

John Hans Tester

Additional Voices (voice)